• International Journal of Technology (IJTech)
  • Vol 7, No 2 (2016)

Characterization of Carbon Nanotubes Synthesized from Hydrocarbon-Rich Flame

Characterization of Carbon Nanotubes Synthesized from Hydrocarbon-Rich Flame

Title: Characterization of Carbon Nanotubes Synthesized from Hydrocarbon-Rich Flame
Win Hon Tan, Siew Ling Lee, Jo Han Ng, William Woei Fong Chong, Cheng Tung Chong

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Published at : 29 Feb 2016
Volume : IJtech Vol 7, No 2 (2016)
DOI : https://doi.org/10.14716/ijtech.v7i2.3284

Cite this article as:

Tan, W.H., Lee, S.L., Ng, J.-H., Chong, W.W.F., Chong, C.T., 2016. Characterization of Carbon Nanotubes Synthesized from Hydrocarbon-Rich Flame. International Journal of Technology. Volume 7(2), pp.343-351

Win Hon Tan Faculty of Mechanical Engineering, Universiti Teknologi Malaysia, 81310 Skudai, Johor, Malaysia
Siew Ling Lee Centre for Sustainable Nanomaterials, Ibnu Sina Institute for Scientific and Industrial Research, Universiti Teknologi Malaysia 81310 Skudai Johor, Malaysia
Jo Han Ng Faculty of Engineering and the Environment, University of Southampton, Malaysia Campus (USMC), 79200 Nusajaya, Johor, Malaysia
William Woei Fong Chong UTM Centre for Low Carbon Transport in cooperation with Imperial College London Universiti Teknologi Malaysia, 81310 Skudai Johor, Malaysia
Cheng Tung Chong UTM Centre for Low Carbon Transport in cooperation with Imperial College London Universiti Teknologi Malaysia, 81310 Skudai Johor, Malaysia
Email to Corresponding Author

Characterization of Carbon Nanotubes Synthesized from Hydrocarbon-Rich Flame

The present study focuses on the characterization of carbon nanotubes (CNTs) synthesized from flame under an atmospheric condition. A laminar flame burner was utilized to establish a rich premixed propane/air flame at the equivalence ratio ? = 1.8–2.2. The flame was impinged on a stainless steel wire mesh coated with nickel (Ni) catalyst to grow CNTs. Distribution and yield of the CNTs on the substrate were quantified. Carbon nanotubes formed on the substrate were harvested and characterized using scanning electron microscopy (SEM), field emission scanning electron microscopy (FESEM), energy dispersive X-ray spectroscopy (EDX), and thermogravimetric analysis (TGA). The FESEM micrograph showed that the CNTs produced were in disarray. The synthesized CNTs were an average of 50–60 nm in diameter while the length of the tubes was in the order of microns. TGA analysis showed that 75% of CNTs were present in the sample and the oxidation temperature was 510°C.

Carbon nanotubes, FESEM, EDX, Flame synthesis, Nickel catalyst


Datsyuk, V., Kalyva, M., Papagelis, K., Parthenios, J., Tasis, D., Siokou, A., Kallitsis, I., Galiotis, C., 2008. Chemical Oxidation of Multiwalled Carbon Nanotubes. Carbon, Volume 46(6), pp. 833–840

Dresselhaus, M.S., Dresselhaus, G., Eklund, P.C., 1996. Science of Fullerenes and Carbon Nanotubes: Their Properties and Applications. Academic Press

Gill, N.S., Taylor, F., Hatfield, W., Parker, W., Fountain, C.S., Bunger, F.L., 1967. Tetrahalo Complexes of Dipositive Metals in the First Transition Series. Inorganic Syntheses, Volume 9, pp. 136–142

Gore, J.P., Sane, A., 2011. Flame Synthesis of Carbon Nanotubes. Carbon Nanotubes-Synthesis, Characterization, Applications, InTech, pp. 122–132

Height, M.J., Howard, J.B., Tester, J.W., Vander Sande, J.B., 2004. Flame Synthesis of Single-Walled Carbon Nanotubes. Carbon, Volume 42(11), pp. 2295–2307

Huang, Z., Wang, D., Wen, J., Sennett, M., Gibson, H., Ren, Z., 2002. Effect of Nickel, Iron, and Cobalt on Growth of Aligned Carbon Nanotubes. Applied Physics A, Volume 74(3), pp. 387–391

Kashir, B., Tabejamaat, S., Baig, M.M. 2012. Experimental Study on Propane/Oxygen and Natural Gas/Oxygen Laminar Diffusion Flames in Diluting and Preheating Conditions. Thermal Science, Volume 16(4), pp. 1043–1053

Kumar, C.S., 2012. Raman Spectroscopy for Nanomaterials Characterization: Springer Science & Business Media

Kumar, M., Ando, Y., 2011. Carbon Nanotube Synthesis and Growth Mechanism: InTech, Open Access Publisher

Lee, C.J., Park, J., Huh, Y., Lee, J.Y., 2001. Temperature Effect on the Growth of Carbon Nanotubes using Thermal Chemical Vapor Deposition. Chemical Physics Letters, Volume 343(1), pp. 33–38

Merchan-Merchan, W., Saveliev, A., Kennedy, L.A., Fridman, A., 2002. Formation of Carbon Nanotubes in Counter-Flow, Oxy-Methane Diffusion Flames without Catalysts. Chemical Physics Letters, Volume 354(1),

pp. 20–24

Shibuta, Y., Suzuki, T., 2010. Melting and Solidification Point of Fcc-metal Nanoparticles with Respect to Particle Size: A Molecular Dynamics Study. Chemical Physics Letters, Volume 498(4), pp. 323–327

Vander Wal, R.L., Hall, L.J., Berger, G.M., 2002. Optimization of Flame Synthesis for Carbon Nanotubes using Supported Catalyst. The Journal of Physical Chemistry B, Volume 106(51), pp. 13122–13132

Vandooren, J., Branch, M., Van Tiggelen, P., 1992. Comparisons of the Structure of Stoichiometric CH4-N2O-Ar and CH4-O2-Ar Flames by Molecular Beam Sampling and Mass Spectrometric Analysis. Combustion and Flame, Volume 90(3), pp. 247–258

Woo, S., Hong, Y., Kwon, O., 2009. Flame-synthesis Limits and Self-catalytic Behavior of Carbon Nanotubes using a Double-faced Wall Stagnation Flow Burner. Combustion and Flame, Volume 156(10), pp. 1983–1992

Zabetta, E.C., Hupa, M., 2005. Gas-born Carbon Particles Generated by Combustion: A Review on the Formation and Relevance. Combustion and Materials Chemistry. ABO AKADEMI, FIN-20500 Åbo, Finland